Amine-bearing hydrocarbon cross-links: Tailoring helix stability, hydrophilicity, and synthetic adaptability in peptides
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초록

This study comprehensively explored the helix-stabilizing effects of amine-bearing hydrocarbon cross-links (ABXs), revealing their context-dependent nature influenced by various structural parameters. Notably, we identified a 9-atom ABX as a robust helix stabilizer, showcasing versatile synthetic adaptability while preserving peptide water solubility. Future investigations are imperative to fully exploit this system's potential and enrich our chemical toolkit for designing innovative peptide-based biomolecules. © 2024 Elsevier Ltd

키워드

Amine cross-linkPeptide drugsPeptide staplingRing-closing metathesisα-Helix
제목
Amine-bearing hydrocarbon cross-links: Tailoring helix stability, hydrophilicity, and synthetic adaptability in peptides
저자
Tran, Duc V.H.Pham, Thanh K.Kim, Young-Woo
DOI
10.1016/j.bmc.2024.117893
발행일
2024-10
유형
Article
저널명
Bioorganic and Medicinal Chemistry
112
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1 ~ 8