A Series of Quinolinol-Based Indium Luminophores: A Rational Design Approach for Manipulating Photophysical Properties
  • Kwak, Sang Woo
  • Kim, Moon Bae
  • Shin, Heuiseok
  • Lee, Ji Hye
  • Hwang, Hyonseok
  • ... Choe, Joong Chul
  • 외 7명
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초록

An approach to the design of a series of quinolinol-based indium complexes that can exhibit different optical properties is proposed. Mono-incorporated (Inq(1) and InMeq(1)), bis-incorporated (InMeq(2)), and tris-incorporated (Inq(3) and InMeq(3)) indium quinolinate complexes have been prepared. These complexes have also been characterized by X-ray crystallography. The photophysical properties of these complexes have also been examined by a combination of experimental and theoretical techniques. The indium complexes with a single quinolinol ligand (Inq(1) and InMeq(1)) showed higher quantum efficiency than those with two or three quinolinate ligands; in particular, InMeq(1) exhibited the highest quantum yield [Phi(PL) = 59% in poly(methyl methacrylate) film]. The insights into the nature of these findings were obtained by the sequential synthesis of the quinolinol-based indium luminophores and a detailed investigation of their structural stability.

키워드

LIGHT-EMITTING-DIODESSUBSTITUTED ALUMINUMCOMPLEXESBLUEELECTROLUMINESCENCEGALLIUMPHOTOLUMINESCENCELUMINESCENCEEMISSIONCRYSTAL
제목
A Series of Quinolinol-Based Indium Luminophores: A Rational Design Approach for Manipulating Photophysical Properties
저자
Kwak, Sang WooKim, Moon BaeShin, HeuiseokLee, Ji HyeHwang, HyonseokRyu, Ji YeonLee, JunseongKim, MinChung, YongseogChoe, Joong ChulKim, YoungjoLee, Kang MunPark, Myung Hwan
DOI
10.1021/acs.inorgchem.9b00802
발행일
2019-06-17
유형
Article
저널명
Inorganic Chemistry
58
12
페이지
8056 ~ 8063