Development of new TAK-285 derivatives as potent EGFR/HER2 inhibitors possessing antiproliferative effects against 22RV1 and PC3 prostate carcinoma cell lines
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초록

Epidermal growth factor receptor (EGFR) and human epidermal growth factor receptor 2 (HER2) protein tyrosine kinases co-expressed in various cancers such as ovarian, breast, colon, and prostate subtypes. Herein, new TAK-285 derivatives (9a-h) were synthesised, characterised, and biologically evaluated as dual EGFR/HER2 inhibitors. Compound 9f exhibited IC50 values of 2.3 nM over EGFR and 234 nM over HER2, which is 38-fold of staurosporine and 10-fold of TAK-285 over EGFR. Compound 9f also showed high selectivity profile when tested over a small kinase panel. Compounds 9a-h showed IC50 values in the range of 1.0-7.3 nM and 0.8-2.8 nM against PC3 and 22RV1 prostate carcinoma cell lines, respectively. Cell cycle analysis, apoptotic induction, molecular docking, dynamics, and MM-GBSA studies confirmed the plausible mechanism(s) of compound 9f as a potent EGFR/HER2 dual inhibitor with an effective antiproliferative action against prostate carcinoma.

키워드

EGFRHER2chemical synthesisapoptosiskinase panelprostate carcinomaBIOLOGICAL EVALUATIONLAPATINIB RESISTANCELUNG-CANCEREGFRDESIGNMUTATIONFAMILYKINASESCOMPLEX
제목
Development of new TAK-285 derivatives as potent EGFR/HER2 inhibitors possessing antiproliferative effects against 22RV1 and PC3 prostate carcinoma cell lines
저자
Son, SeohyunElkamhawy, AhmedGul, Anam RanaAl-Karmalawy, Ahmed A.Alnajjar, RadwanAbdeen, AhmedIbrahim, Samah F.Alshammari, Saud O.Alshammari, Qamar A.Choi, Won JunPark, Tae JungLee, Kyeong
DOI
10.1080/14756366.2023.2202358
발행일
2023-12
유형
Article
저널명
Journal of Enzyme Inhibition and Medicinal Chemistry
38
1
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1 ~ 17