Base-Catalyzed One-Pot Synthesis of Indolizine-1-carboxylates Tethered to 2-Aroyl Benzofurans and Benzothiophenes
  • Lee, Juyoung
  • Ahn, Sooseong
  • Eom, Kihyeon
  • Park, Younggeun
  • Lee, Kyeong
  • 외 2명
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초록

Herein, we report a base-catalyzed one-pot synthesis of indolizine-1-carboxylates tethered to 2-aroyl benzofurans and benzothiophenes from 2-pyridin-2-ylacetates, DMF-DMA, and 2-aroyl-benzofuran/benzothiophene-3-methyl bromides. This protocol provides access to diverse indolizine derivatives in moderate to good yields under simple conditions. A broad range of substituents on both the benzofuran/benzothiophene and pyridine-2-ylacetate components was tolerated well, and gram-scale synthesis was achieved without chromatographic purification. In addition, postsynthetic Suzuki coupling of the bromine-containing products enabled the construction of highly conjugated indolizine-benzofuran architectures.

키워드

BIOACTIVITYINDOLIZINES
제목
Base-Catalyzed One-Pot Synthesis of Indolizine-1-carboxylates Tethered to 2-Aroyl Benzofurans and Benzothiophenes
저자
Lee, JuyoungAhn, SooseongEom, KihyeonPark, YounggeunLee, KyeongJalani, Hitesh B.Choi, Yongseok
DOI
10.1021/acs.joc.6c00082
발행일
2026-04
유형
Article
저널명
Journal of Organic Chemistry
91
16
페이지
5713 ~ 5717